This collection consists of seven videotapes recorded at Virginia Polytechnic Institute and State University (or Virginia Tech) in August 1991. The tapes contain interviews with six nuclear pioneers: Sigvard Eklund, Bertrand Goldschmidt, Robert E. Marshak, Glenn T. Seaborg, Gerald F. Tape, and Herbert F. York. Five of the tapes cover four main topics in nuclear history during the period from about 1945 through 1965: weapons and the arms race, civilian vs. military control in post-World War II United States, peaceful uses of the atom and basic research, and international perspectives on research, development, and cooperation. Two additional tapes cover a two-hour public round table where the pioneers were interviewed by Jerry Bishop of the Wall Street Journal, Gloria Lubkin of Physics Today, Albert Moyer of Virginia Tech, and Paul Torgersen of Virginia Tech.

In addition to the tapes, the collection includes supporting documentation and papers for the sessions such as event cards, partial transcripts, and planning information.