The Charles S. Worley, Jr., Collection consist of architectural drawings of designs by Worley, done from the mid-1950s to the early 1960s, with several designs undated. The collection also includes a small group of photographs and negatives of Worley and his own residence in Blacksburg, as well as an extensive collection of slides documenting Worley's student and professional work, work of his students, his travels, nature, and images that were likely used as part of lectures.

A spreadsheet inventory of the slide topics, based on Worley's original organization, is available online.